4,5,9,10-Pyrenetetrone, 2,7-bis(1,1-dimethylethyl)-

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CAS: 190843-93-7
MF: C24H22O4
MW: 374.42908
Synonyms: 4,5,9,10-Pyrenetetrone, 2,7-bis(1,1-dimethylethyl)-

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YanXiang Cheng

Changchun Institute of Applied Chemistry, Chinese Academy of Sciences
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Lixiang Wang

Chinese Academy of Sciences
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Xian-He Bu

Nankai University
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Ze Chang

Nankai University
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Co-reporter: Le-Le Yang, Xiu-Ming Liu, Kun Liu, Huan Liu, Fang-Yao Zhao, Wen-Juan Ruan, Yue Li, Ze Chang, Xian-He Bu
pp: 278-283
Publication Date(Web):1 October 2014
DOI: 10.1016/j.talanta.2014.04.046
•A sensor (1) with quadrapyridyl type receptor and large chromophore was obtained.•1 exhibit sensitive off-on fluorescent response to Cd2+ in aqueous media.•The response of 1 to Cd2+ is immune to the interference of other metal cations.•1 is highly biocompatible and was used to the in vivo Cd2+ imaging in living cells.By retaining the quadrapyridyl receptor of polypyridylhexaazatriphenylene (a Cd2+ sensor reported by us) and extending its chromophoric group with pyrene, a chemical sensor (1) was designed and synthesized in this work. This sensor exhibit selective off-on fluorescence response to Cd2+ over other metal ions, and the detection limit is as low as 0.02 μM. The Cd2+ sensing of 1 has high water toleration and can be carried out in the media with the water content up to 70%. Additionally, 1 was successfully applied to the in vivo imaging of intracellular Cd2+ in living HaLa cells, and showed low cytotoxicity and cell membrane permeability in these experiments. These results suggest that 1 has potential application in the Cd2+ analysis of environmental and biological samples.A polypyridyl-pyrene based chemical sensor showed selective off-on fluorescence response to Cd2+ in aqueous media and was successfully applied to the in vivo imaging of Cd2+ in living cells.Image for unlabelled figure

Yue Li

Nankai University
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Co-reporter: Le-Le Yang, Xiu-Ming Liu, Kun Liu, Huan Liu, Fang-Yao Zhao, Wen-Juan Ruan, Yue Li, Ze Chang, Xian-He Bu
pp: 278-283
Publication Date(Web):1 October 2014
DOI: 10.1016/j.talanta.2014.04.046
•A sensor (1) with quadrapyridyl type receptor and large chromophore was obtained.•1 exhibit sensitive off-on fluorescent response to Cd2+ in aqueous media.•The response of 1 to Cd2+ is immune to the interference of other metal cations.•1 is highly biocompatible and was used to the in vivo Cd2+ imaging in living cells.By retaining the quadrapyridyl receptor of polypyridylhexaazatriphenylene (a Cd2+ sensor reported by us) and extending its chromophoric group with pyrene, a chemical sensor (1) was designed and synthesized in this work. This sensor exhibit selective off-on fluorescence response to Cd2+ over other metal ions, and the detection limit is as low as 0.02 μM. The Cd2+ sensing of 1 has high water toleration and can be carried out in the media with the water content up to 70%. Additionally, 1 was successfully applied to the in vivo imaging of intracellular Cd2+ in living HaLa cells, and showed low cytotoxicity and cell membrane permeability in these experiments. These results suggest that 1 has potential application in the Cd2+ analysis of environmental and biological samples.A polypyridyl-pyrene based chemical sensor showed selective off-on fluorescence response to Cd2+ in aqueous media and was successfully applied to the in vivo imaging of Cd2+ in living cells.Image for unlabelled figure

Wei Huang

Nanjing University
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Eric Meggers

Philipps-Universit?t Marburg
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Klaus Muellen

Max Planck Institute for Polymer Research
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Wojciech Pisula

Max Planck Institute for Polymer Research
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Denis Andrienko

Max Planck Institute for Polymer Research
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